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Ironcobaltnickel trimetal phosphides as high-performance electrocatalysts for overall water splitting.Herein, we fabricate an NP-codoped FeCoNi-containing graphene-based material by deriving metalorganic frameworks (MOFs).The homogeneous dispersion of tri-metallic FeCoNi in the MOF-derived carbon materials favors the formation of heterojunctions between the resulted different phosphides, which speed up electron transfer and improve the electrocatalytic properties.The graphene support can efficiently protect the phosphides from degradation during the catalytic process.
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